Possible quadrupole-order-driven commensurate-incommensurate phase transition in B20 CoGe

نویسندگان

چکیده

The B20-type cobalt germanide CoGe was investigated by measuring the specific heat, resistivity, and $^{59}$Co nuclear magnetic resonance (NMR). We observed a phase transition at $T_Q=13.7$ K, evidenced very narrow peak of heat sharp changes spin-spin ($T_2^{-1}$) spin-lattice ($T_1^{-1}$) relaxation rates. fact that entropy release is extremely small Knight shift almost independent temperature down to low temperatures as anticipated in paramagnetic metal indicates $T_Q$ non-magnetic origin. In addition, we detected crossover scale $T_0\sim30$ K below which resistivity NMR linewidth increase, $T_1^{-1}$ progressively distributed space, is, static dynamical spatial inhomogeneity develops. While order parameter for remains an open question, group-theoretical analysis suggests finite electric quadrupole density arising from local site symmetry sites could drive crystal lowering P2$_1$3 commensurate R3 with incommensurate wavevector, fairly well accounts transition. quadrupole-order-driven commensurate-incommensurate may be another remarkable phenomenon structural chirality inherent noncentrosymmetric B20 family.

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ژورنال

عنوان ژورنال: Physical review

سال: 2022

ISSN: ['0556-2813', '1538-4497', '1089-490X']

DOI: https://doi.org/10.1103/physrevb.105.165132